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2022-03-04
摘要翻译:
光合作用的整个过程包括两个主要阶段,即光和暗作用:光能被叶绿素分子吸收并转移到再生NADH和ATP,然后驱动Calvin-Benson循环合成糖。要想通过人工光合作用合成糖,关键之一是经济地再生ATP,提高暗反应效率。本文提出了9种暗反应途径,仅用氢气或电来驱动NADH,提高了暗反应的效率,结合太阳能光伏或太阳能氢技术,人工光合作用的总效率可达30%,是自然光合作用的几十倍。其中,以CO2和H2为原料化学合成甲醛,不需要NADH和ATP,通过9种酶高效合成糖,易于大规模生产,而且糖可以通过酶高效转化为载能氢,是一种很好的能量载体。
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英文标题:
《Synthesis of Sugar and fixation of CO2 through Artificial Photosynthesis
  driving by Hydrogen or Electricity》
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作者:
Weidong Huang
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最新提交年份:
2010
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分类信息:

一级分类:Physics        物理学
二级分类:Chemical Physics        化学物理学
分类描述:Experimental, computational, and theoretical physics of atoms, molecules, and clusters - Classical and quantum description of states, processes, and dynamics; spectroscopy, electronic structure, conformations, reactions, interactions, and phases. Chemical thermodynamics. Disperse systems. High pressure chemistry. Solid state chemistry. Surface and interface chemistry.
原子、分子和团簇的实验、计算和理论物理-状态、过程和动力学的经典和量子描述;光谱学,电子结构,构象,反应,相互作用和相。化学热力学。分散系统。高压化学。固态化学。表面和界面化学。
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一级分类:Physics        物理学
二级分类:Biological Physics        生物物理学
分类描述:Molecular biophysics, cellular biophysics, neurological biophysics, membrane biophysics, single-molecule biophysics, ecological biophysics, quantum phenomena in biological systems (quantum biophysics), theoretical biophysics, molecular dynamics/modeling and simulation, game theory, biomechanics, bioinformatics, microorganisms, virology, evolution, biophysical methods.
分子生物物理、细胞生物物理、神经生物物理、膜生物物理、单分子生物物理、生态生物物理、生物系统中的量子现象(量子生物物理)、理论生物物理、分子动力学/建模与模拟、博弈论、生物力学、生物信息学、微生物、病毒学、进化论、生物物理方法。
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一级分类:Quantitative Biology        数量生物学
二级分类:Other Quantitative Biology        其他定量生物学
分类描述:Work in quantitative biology that does not fit into the other q-bio classifications
不适合其他q-bio分类的定量生物学工作
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英文摘要:
  The overall process of photosynthesis consists of two main phases, the so-called light and dark eactions: light energy is absorbed by chlorophyll molecules and transferred to regenerate NADH and ATP, then drive Calvin-Benson cycle to synthesize sugar. In order to synthesize sugar through artificial photosynthesis, one of the key is to regenerate ATP economically and improve the efficiency of dark reactions. Here 9 kinds of dark reaction pathways are proposed, which only NADH is regenearated from hydrogen or electricity for driving, the efficiency of dark reactions is improved, combined with solar photovoltaic or solar hydrogen technology, the total efficiency of artificial photosynthesis can reach 30%, several ten times more than natural photosynthesis. One of them, to use chemical synthesis of formaldehyde from CO2 and H2, no NADH and ATP is need, to synthesize sugar efficiently through 9 enzymes, so it will be easier to produce in large scale, and the sugar will be a good energy carrier as the sugar can be efficiently converted to energy carrier hydrogen through enzymes.
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PDF链接:
https://arxiv.org/pdf/1009.0310
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