摘要翻译:
在准弹性He原子散射实验中,Na原子在Cu(001)上的扩散复盖率达20%时,用相互作用单吸附质近似描述了相互作用表面的活化扩散。这种近似基本上包括求解带有两个噪声源和摩擦的标准朗之万方程:高斯白噪声和白散粒噪声,前者考虑了与基底的摩擦,后者描述了模拟吸附质-吸附质碰撞的碰撞摩擦。在200K和300K两个表面温度下,准弹性峰的展宽与实验数据非常吻合。
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英文标题:
《Stochastic theory of lineshape broadening in quasielastic He atom
scattering with interacting adsorbates》
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作者:
R. Martinez-Casado, J. L. Vega, A. S. Sanz, S. Miret-Artes
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最新提交年份:
2008
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分类信息:
一级分类:Physics 物理学
二级分类:Statistical Mechanics 统计力学
分类描述:Phase transitions, thermodynamics, field theory, non-equilibrium phenomena, renormalization group and scaling, integrable models, turbulence
相变,热力学,场论,非平衡现象,重整化群和标度,可积模型,湍流
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一级分类:Physics 物理学
二级分类:Materials Science 材料科学
分类描述:Techniques, synthesis, characterization, structure. Structural phase transitions, mechanical properties, phonons. Defects, adsorbates, interfaces
技术,合成,表征,结构。结构相变,力学性质,声子。缺陷,吸附质,界面
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一级分类:Physics 物理学
二级分类:Quantum Physics 量子物理学
分类描述:Description coming soon
描述即将到来
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英文摘要:
The activated surface diffusion of interacting adsorbates is described in terms of the so-called interacting single adsorbate approximation, which is applied to the diffusion of Na atoms on Cu(001) for coverages up to 20% in quasielastic He atom scattering experiments. This approximation essentially consists of solving the standard Langevin equation with two noise sources and frictions: a Gaussian white noise accounting for the friction with the substrate, and a white shot noise characterized by a collisional friction simulating the adsorbate-adsorbate collisions. The broadenings undergone by the quasielastic peak are found to be in very good agreement with the experimental data reported at two surface temperatures 200 and 300 K.
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PDF链接:
https://arxiv.org/pdf/710.3266