摘要翻译:
在快速重离子辐照下,从包埋金纳米粒子溅射出的Au团簇中,发现了两个关于$n$-原子团簇尺寸分布的指数:$y(n)\sim n^{-\delta}$。对于尺寸小于12.5nm的小团簇,$\delta$为3/2,这可以归结为一个与尺寸无关的稳态聚集过程。对于较大的团簇,$\delta值建议为7/2,这可能来自于向另一个稳态的动力学转变,在此稳态中聚集和蒸发速率与尺寸有关。在目前的情况下,观察到的衰变指数不支持任何发生热力学液-气型相变的可能性,从而导致团簇的形成。
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英文标题:
《Observation of a Universal Aggregation Mechanism and a Possible Phase
Transition in Au Sputtered by Swift Heavy Ions》
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作者:
P. K. Kuiri, B. Joseph, H. P. Lenka, G. Sahu, J. Ghatak, D. Kanjilal,
and D. P. Mahapatra
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最新提交年份:
2009
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分类信息:
一级分类:Physics 物理学
二级分类:Materials Science 材料科学
分类描述:Techniques, synthesis, characterization, structure. Structural phase transitions, mechanical properties, phonons. Defects, adsorbates, interfaces
技术,合成,表征,结构。结构相变,力学性质,声子。缺陷,吸附质,界面
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一级分类:Physics 物理学
二级分类:Statistical Mechanics 统计力学
分类描述:Phase transitions, thermodynamics, field theory, non-equilibrium phenomena, renormalization group and scaling, integrable models, turbulence
相变,热力学,场论,非平衡现象,重整化群和标度,可积模型,湍流
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英文摘要:
Two exponents, $\delta$, for size distribution of $n$-atom clusters, $Y(n)\sim n^{-\delta}$, have been found in Au clusters sputtered from embedded Au nanoparticles under swift heavy ion irradiation. For small clusters, below 12.5 nm in size, $\delta$ has been found to be 3/2, which can be rationalized as occurring from a steady state aggregation process with size independent aggregation. For larger clusters, a $\delta$ value of 7/2 is suggested, which might come from a dynamical transition to another steady state where aggregation and evaporation rates are size dependent. In the present case, the observed decay exponents do not support any possibility of a thermodynamic liquid-gas type phase transition taking place, resulting in cluster formation.
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PDF链接:
https://arxiv.org/pdf/802.2494